TY - JOUR T1 - Emission Spectrum of Two-Level Single Molecule via Photon Counting Statistics AU - Peng , Yonggang JO - Journal of Atomic and Molecular Sciences VL - 4 SP - 200 EP - 206 PY - 2016 DA - 2016/07 SN - 7 DO - http://doi.org/10.4208/jams.052316.082216a UR - https://global-sci.org/intro/article_detail/jams/8159.html KW - Two-Level System, Emission Spectrum, Generating Function. AB -

In this paper, we introduce a new way to obtain the emission spectrum of single molecule driven by external field. A virtual probe field is introduced to simulate the vacuum field, which causes the spontaneous emission phenomena of the excited single molecule. The statistical properties of the emission photons caused by the virtual probe field could be used to obtain the emission spectrum of the single molecule system. The results demonstrate the well-known Mollow triplet splitting phenomenon as the single molecule is driven by strong external field.The abstract should provide a brief summary of the main findings of the paper.