A 2-D Kinetic Theory for Flows of Monodomain Polymer-Rod Nanocomposites

A 2-D Kinetic Theory for Flows of Monodomain Polymer-Rod Nanocomposites

Year:    2010

Communications in Computational Physics, Vol. 7 (2010), Iss. 2 : pp. 250–282

Abstract

We merge classical kinetic theories [M. Doi and S. F. Edwards, The Theory of Polymer Dynamics, 1986] for viscous dispersions of rigid rods, extended to semi-flexibility [A. R. Khokhlov and A. N. Semenov, Macromolecules, 17 (1984), pp. 2678-2685], and for Rouse flexible chains to model the hydrodynamics of polymer nano-rod composites (PNCs). A mean-field potential for the polymer-rod interface provides the key coupling between the two phases. We restrict this first study to two-dimensional conformational space. We solve the coupled set of Smoluchowski equations for three benchmark experiments. First we explore how rod semi-flexibility and the polymerrod interface alter the Onsager equilibrium phase diagram. Then we determine monodomain phase behavior of PNCs for imposed simple elongation and shear, respectively. These results inform the effects that each phase has on the other as parametric strengths of the interactions are varied in the context of the most basic rheological experiments.

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Journal Article Details

Publisher Name:    Global Science Press

Language:    English

DOI:    https://doi.org/10.4208/cicp.2009.08.204

Communications in Computational Physics, Vol. 7 (2010), Iss. 2 : pp. 250–282

Published online:    2010-01

AMS Subject Headings:    Global Science Press

Copyright:    COPYRIGHT: © Global Science Press

Pages:    33

Keywords:   

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